The Source of Green Light Emission Determined from a Heavy-Ion Storage Ring Experiment
D. Kella,
L. Vejby-Christensen,
P. J. Johnson,
H. B. Pedersen,
L. H. Andersen
*
The final electronic states of oxygen atoms formed by dissociative
recombination of O2+ with cold electrons have
been measured by an imaging technique at a heavy-ion storage ring. The
3P, 1D, and
1S quantum yield for O2+
in the vibrational ground level was found to be 0.86, 1.09, and 0.05, respectively. The yield of the 1S state, which
is responsible for the 5577 angstrom green light from upper planetary
atmospheres, was more than an order of magnitude larger than the
theoretical value used in atmospheric models. The results may help
refine the models of the chemistry and dynamics of the ionosphere and
provide guidance for further quantum-chemistry calculations.
Institute of Physics and Astronomy, University of Aarhus, DK 8000, Aarhus C, Denmark.
*
To whom correspondence should be addressed. E-mail:
lha{at}dfi.aau.dk