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Science 28 July 2006:
Vol. 313. no. 5786, pp. 502 - 504
DOI: 10.1126/science.1129198

Reports

Second-Harmonic Generation from Magnetic Metamaterials

Matthias W. Klein,1,2 Christian Enkrich,1,2 Martin Wegener,1,2,3 Stefan Linden1,2,3*

We observe second-harmonic generation from metamaterials composed of split-ring resonators excited at 1.5-micrometer wavelength. Much larger signals are detected when magnetic-dipole resonances are excited, as compared with purely electric-dipole resonances. The experiments are consistent with calculations based on the magnetic component of the Lorentz force exerted on metal electrons—an intrinsic second-harmonic generation mechanism that plays no role in natural materials. This unusual mechanism becomes relevant in our work as a result of the enhancement and the orientation of the local magnetic fields associated with the magnetic-dipole resonances of the split-ring resonators.

1 Institut für Angewandte Physik, Universität Karlsruhe (TH), Wolfgang-Gaede-Straße 1, D-76131 Karlsruhe, Germany.
2 DFG-Center for Functional Nanostructures (CFN), Universität Karlsruhe (TH), D-76128 Karlsruhe, Germany.
3 Institut für Nanotechnologie, Forschungszentrum Karlsruhe in der Helmholtz-Gemeinschaft, D-76021 Karlsruhe, Germany.

* To whom correspondence should be addressed. E-mail: stefan.linden{at}physik.uni-karlsruhe.de

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Science. ISSN 0036-8075 (print), 1095-9203 (online)