Probing and Controlling the Bonds of an Artificial Molecule
Alexander W. Holleitner,1*
Robert H. Blick,1
Andreas K. Hüttel,1
Karl Eberl,2
Jörg P. Kotthaus1
We demonstrate how molecular quantum states of coupled
semiconductor quantum dots are coherently probed and manipulated in transport experiments. The applied method probes quantum states by the
virtual cotunneling of two electrons and hence resolves the sequences
of molecular states simultaneously. This result is achieved by weakly
probing the quantum system through parallel contacts to its
constituting quantum dots. The overlap of the dots' wave functions
and, in turn, the splitting of molecular states are adjusted by the
direct influence of coupling electrodes.
1 Center for NanoScience and Sektion Physik,
Ludwig-Maximilians-Universität, Geschwister-Scholl-Platz 1, 80539 München, Germany.
2 Max-Planck-Institut
für Festkörperforschung, Heisenbergstrasse 1, 70569 Stuttgart, Germany.
*
To whom correspondence should be addressed. E-mail:
Alex.Holleitner{at}physik.uni-muenchen.de