Ultrafast Manipulation of Electron Spin Coherence
J. A. Gupta,1
R. Knobel,2
N. Samarth,2
D. D. Awschalom1*
A technique is developed with the potential for coherent
all-optical control over electron spins in semiconductors on
femtosecond time scales. The experiments show that optical
"tipping" pulses can enact substantial rotations of electron spins
through a mechanism dependent on the optical Stark effect. These
rotations were measured as changes in the amplitude of spin precession
after optical excitation in a transverse magnetic field and approach
/2 radians. A prototype sequence of two tipping pulses indicates
that the rotation is reversible, a result that establishes the coherent
nature of the tipping process.
1 Department of Physics, University of
California, Santa Barbara, CA 93106, USA.
2 Department of Physics, The Pennsylvania State
University, University Park, PA 16802, USA.
*
To whom correspondence should be addressed. E-mail:
awsch{at}physics.ucsb.edu