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Originally published in Science Express on 10 May 2001
Science 29 June 2001:
Vol. 292. no. 5526, pp. 2453 - 2458
DOI: 10.1126/science.1056649

Research Articles

Extremely Large Variations of Atmospheric 14C Concentration During the Last Glacial Period

J. Warren Beck,1* David A. Richards,23* R. Lawrence , Edwards,3 Bernard W. Silverman,4 Peter L. Smart,2 Douglas J. Donahue,1 Sofia Hererra-Osterheld,1 George. S. Burr,1 Leal Calsoyas,1 A. J. Timothy , Jull,1 Dana Biddulph1

A long record of atmospheric 14C concentration, from 45 to 11 thousand years ago (ka), was obtained from a stalagmite with thermal-ionization mass-spectrometric 230Th and accelerator mass-spectrometric 14C measurements. This record reveals highly elevated Delta 14C between 45 and 33 ka, portions of which may correlate with peaks in cosmogenic 36Cl and 10Be isotopes observed in polar ice cores. Superimposed on this broad peak of Delta 14C are several rapid excursions, the largest of which occurs between 44.3 and 43.3 ka. Between 26 and 11 ka, atmospheric Delta 14C decreased from ~700 to ~100 per mil, modulated by numerous minor excursions. Carbon cycle models suggest that the major features of this record cannot be produced with solar or terrestrial magnetic field modulation alone but also require substantial fluctuations in the carbon cycle.

1 NSF-Arizona Accelerator Mass Spectrometry Facility, Department of Physics, University of Arizona, Tucson, AZ 85721, USA.
2 School of Geographical Sciences, University of Bristol, Bristol, BS8 1SS, UK.
3 Minnesota Isotope Laboratory, Department of Geology and Geophysics, University of Minnesota, Minneapolis, MN 55455, USA.
4 School of Mathematics, University of Bristol, Bristol, BS8 1TW, UK.
*   To whom correspondence should be addressed. E-mail: wbeck{at}physics.arizona.edu, David.Richards{at}bristol.ac.uk


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Science. ISSN 0036-8075 (print), 1095-9203 (online)