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Science 1 December 2000:
Vol. 290. no. 5497, pp. 1739 - 1742
DOI: 10.1126/science.290.5497.1739

Reports

Self-Mode-Locking of Quantum Cascade Lasers with Giant Ultrafast Optical Nonlinearities

Roberto Paiella,1* Federico Capasso,1 Claire Gmachl,1 Deborah L. Sivco,1 James N. Baillargeon,1 Albert L. Hutchinson,1 Alfred Y. Cho,1 H. C. Liu2

We report on the generation of picosecond self-mode-locked pulses from midinfrared quantum cascade lasers, at wavelengths within the important molecular fingerprint region. These devices are based on intersubband electron transitions in semiconductor nanostructures, which are characterized by some of the largest optical nonlinearities observed in nature and by picosecond relaxation lifetimes. Our results are interpreted with a model in which one of these nonlinearities, the intensity-dependent refractive index of the lasing transition, creates a nonlinear waveguide where the optical losses decrease with increasing intensity. This favors the generation of ultrashort pulses, because of their larger instantaneous intensity relative to continuous-wave emission.

1 Bell Laboratories, Lucent Technologies, 600 Mountain Avenue, Murray Hill, NJ 07974, USA.
2 Institute for Microstructural Sciences, National Research Council, Ottawa, Ontario, K1A 0R6, Canada.
*   To whom correspondence should be addressed. E-mail: robertop{at}lucent.com


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Science. ISSN 0036-8075 (print), 1095-9203 (online)