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Articles
Controlled Deposition, Soft Landing, and Glass Formation in Nanocluster-Surface Collisions
1 School of Physics, Georgia Institute of Technology, Atlanta, GA 30332
Molecular dynamics simulations have been used to investigate the dynamics and redistribution of energy during the impact of a nanocrystal with adsorbed liquid films. Although impact of a 32-molecule NaCl cluster on a solid surface at 3 kilometers per second leads to melting, disordering, fragmentation, and rebounding, the same size cluster colliding with a liquid neon film transfers its energy efficiently to the liquid for a controlled soft landing. Impact on a higher density film (argon) leads to rapid attenuation of the cluster velocity, accompanied by fast heating. Subsequent disordering, melting, and fast cooling by evaporation of argon quench the cluster to a glassy state. These results suggest a method for the controlled growth of nanophase materials. Accepted on March 23, 1993
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Science. ISSN 0036-8075 (print), 1095-9203 (online)