Submitted on November 9, 2001
Accepted on January 8, 2002
Magnetic Resonant Mode in the Single-Layer High-Temperature Superconductor Tl2Ba2CuO6+
H. He 1,
P. Bourges 2,
Y. Sidis 2,
C. Ulrich 1,
L. P. Regnault 3,
S. Pailhès 2,
N. S. Berzigiarova 4,
N. N. Kolesnikov 4,
B. Keimer 1*
1 Max-Planck-Institut für Festkörperforschung, 70569 Stuttgart, Germany.
2 Laboratoire Léon Brillouin, CEA-CNRS, CE Saclay, 91191 Gif sur Yvette, France.
3 CEA Grenoble, Département de Recherche Fondamentale sur la Matière Condensée, 38054 Grenoble cedex 9, France.
4 Institute of Solid State Physics, Russian Academy of Science, Chernogolovka, 142432 Russia.
* To whom correspondence should be addressed. E-mail: b.keimer{at}fkf.mpg.de.
An unusual spin excitation mode observed by neutron scattering has inspired numerous theoretical studies of the interplay between charged quasiparticles and collective spin excitations in the copper oxide high temperature superconductors. The mode has thus far only been observed in materials with crystal structures consisting of copper oxide bilayers, and it is notably absent in the single-layer compound La2-xSrxCuO4+
. Neutron scattering data now show that the mode is present in Tl2Ba2CuO6+
, a single-layer compound with Tc ~ 90 K, thus demonstrating that it is a generic feature of the copper oxide superconductors, independent of the layer sequence. This restricts the theoretical models for the origin of the resonant mode and its role in the mechanism of high temperature superconductivity.